The best CV music IMO is Belmont's revenge soundtrack; no other game will ever have the gothic-yet-not-cheesy-but-classy tone of that whole game, every track is not just good VG music, just change the 6bit chiptone for a piano and you have some masterful solo pieces. That's the unbeateable soundtrack for me and second place is LoS' (Third is Curse of Darkness, great stuff there too)